2001–2015: Films and music documentaries
Crowe followed Almost Famous with the psychological thriller Vanilla Sky in 2001. The film, starring Tom Cruise, Penélope Cruz, and Cameron Diaz, received mixed reviews, but grossed $100.6 million at the US box office, making it his second highest grossing directorial effort behind Jerry Maguire (1996). Vanilla Sky is a remake of Alejandro Amenabar's 1997 Spanish film Abre Los Ojos (Open Your Eyes). Sofia is played by Cruz in both Amenabar's movie and Crowe's remake.
In 2005, Crowe directed the romantic tragicomedy Elizabethtown, starring Orlando Bloom and Kirsten Dunst, which opened to mixed reviews, scoring 45 on Metacritic, the same as Vanilla Sky.
In November 2009, Crowe began filming a behind-the-scenes look at the creation of the album The Union, a collaboration between musicians Elton John and Leon Russell produced by T-Bone Burnett. The documentary features musicians Neil Young, Brian Wilson, Booker T. Jones, steel guitarist Robert Randolph, Don Was and a 10-piece gospel choir who all appear on the album with John and Russell. Musician Stevie Nicks and John's longtime lyricist Bernie Taupin also appear. On March 2, 2011, the documentary was announced to open the 2011 Tribeca Film Festival.
In an interview with Pearl Jam on March 9, 2009, bassist Jeff Ament said that their manager Kelly "has had the idea to do a 20-year anniversary retrospective movie so he's been on board with [film director] Cameron Crowe for the last few years." The band's guitarist Mike McCready said in March, "We are just in the very early stages of that, . . . starting to go through all the footage we have, and Cameron's writing the treatment." Preliminary footage was shot in June 2010. A trailer for the movie Pearl Jam Twenty, which featured Pearl Jam frontman Eddie Vedder choosing between three permanent markers in a shop before turning to the camera and saying "Three's good... Twenty is better", was shown before select movies at the 2011 BFI London Film Festival. The film premiered at the 2011 Toronto International Film Festival and had an accompanying book and soundtrack.
With production on the film Aloha delayed, Crowe set his next feature, the family comedy-drama We Bought a Zoo, based on Benjamin Mee's memoir of the same name. He collaborated with The Devil Wears Prada writer Aline Brosh McKenna on the screenplay. The book's story follows Mee, who buys and moves into a dilapidated zoo (now Dartmoor Zoological Park) in the English countryside. Looking for a fresh start along with his seven-year-old daughter and his troubled 14-year-old son, he hopes to refurbish the zoo, run it, and give his children what he calls an "adventure". Crowe changed the location to the United States. The film received a wide release on December 23, 2011, by 20th Century Fox, and starred Matt Damon and Scarlett Johansson. It received mixed reviews. The music is by Jonsi.
It was announced in early June 2008 that Crowe would return to write and direct his seventh feature film, initially titled Deep Tiki and Volcano Romance, set to star Ben Stiller and Reese Witherspoon, and to be released by Columbia Pictures. Filming was expected to begin in January 2009, but this was postponed.
The project resurfaced in 2013. Bradley Cooper, Emma Stone, Rachel McAdams, Alec Baldwin, Bill Murray, John Krasinski, and Danny McBride joined the cast; filming began in Hawaii in September 2013. The film's final title was Aloha and it was released on May 29, 2015, by Sony Pictures to poor reviews.